Ultrafast spectroscopies have become an important tool for elucidating the microscopic description and dynamical properties of quantum materials. In particular, by tracking the dynamics of nonthermal electrons, a material’s dominant scattering processes can be revealed. Here, we present a method for extracting the electron-phonon coupling strength in the time domain, using time- and angle-resolved photoemission spectroscopy (TR-ARPES). This method is demonstrated in graphite, where we investigate the dynamics of photoinjected electrons at the
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point, detecting quantized energy-loss processes that correspond to the emission of strongly coupled optical phonons. We show that the observed characteristic time scale for spectral weight transfer mediated by phonon-scattering processes allows for the direct quantitative extraction of electron-phonon matrix elements for specific modes. -
Matt, C. E. ; Fatuzzo, C. G. ; Sassa, Y. ; Månsson, M. ; Fatale, S. ; Bitetta, V. ; Shi, X. ; Pailhès, S. ; Berntsen, M. H. ; Kurosawa, T. ; et al ( , Physical Review B)